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Here, we investigate the local electronic structures of the ilmenite iridates $A\\mathrm{IrO}_3$ ($A = \\mathrm{Mg}, \\mathrm{Zn}, \\mathrm{Cd}$) and the hyperhoneycomb $\\beta\\text{-}\\mathrm{ZnIrO}_3$ using Ir $L_3$-edge resonant inelastic x-ray scattering (RIXS). Multiplet analysis of the RIXS spectra reveals a systematic evolution of the crystal field and intraionic interaction param","authors_text":"Hakuto Suzuki, Hiroko Aruga Katori, Kenji Ishii, Yuya Haraguchi","cross_cats":[],"headline":"Local multiplet parameters match in ilmenite and hyperhoneycomb ZnIrO3, showing lattice structure alone controls their distinct magnetic states.","license":"http://creativecommons.org/licenses/by/4.0/","primary_cat":"cond-mat.str-el","submitted_at":"2026-04-10T04:02:58Z","title":"Evolution of crystal field and intraionic interactions in the ilmenite $A$IrO$_3$ ($A$ = Mg, Zn, Cd) and hyperhoneycomb $\\beta$-ZnIrO$_3$"},"references":{"count":34,"internal_anchors":0,"resolved_work":34,"sample":[{"cited_arxiv_id":"","doi":"","is_internal_anchor":false,"ref_index":1,"title":"Kitaev, Anyons in an exactly solved model and be- yond, Ann","work_id":"2658fcad-cd09-449b-b1ce-5bf63ad69dfb","year":2006},{"cited_arxiv_id":"","doi":"","is_internal_anchor":false,"ref_index":2,"title":"L. Savary and L. Balents, Quantum spin liquids: a re- view, Rep. Prog. Phys. 80, 016502 (2017)","work_id":"7c6ca184-bacb-4930-8d28-b2f7653d493e","year":2017},{"cited_arxiv_id":"","doi":"","is_internal_anchor":false,"ref_index":3,"title":"G. Jackeli and G. Khaliullin, Mott insulators in the strong spin-orbit coupling limit: From Heisen- berg to a quantum compass and Kitaev models, Phys. Rev. Lett. 102, 017205 (2009)","work_id":"58180566-cbca-410f-826f-3b3f1efccf49","year":2009},{"cited_arxiv_id":"","doi":"","is_internal_anchor":false,"ref_index":4,"title":"J. G. Rau, E. K.-H. Lee, and H.-Y. Kee, Spin- orbit physics giving rise to novel phases in cor- related systems: Iridates and related materials, Annu. Rev. Condens. Matter Phys. 7, 195 (2016)","work_id":"c1af3738-e88e-413c-9d38-31bcb18cdaa3","year":2016},{"cited_arxiv_id":"","doi":"","is_internal_anchor":false,"ref_index":5,"title":"M. Hermanns, I. Kimchi, and J. Knolle, Physics of the Kitaev model: Fractionalization, dy- namic correlations, and material connections, Annu. Rev. Condens. Matter Phys. 9, 17 (2018)","work_id":"35c814d0-0636-4abc-9cec-5e6773fa99f7","year":2018}],"snapshot_sha256":"9d92aff8eddbc77d81f1941d92d9115211f69f5eafe4c46956c2cbf20f626065"},"source":{"id":"2604.08934","kind":"arxiv","version":1},"verdict":{"created_at":"2026-05-10T17:56:44.245024Z","id":"871d16fb-ffa1-4ab5-b524-a986e6da2bf9","model_set":{"reader":"grok-4.3"},"one_line_summary":"RIXS multiplet analysis finds increasing trigonal distortion with larger A-site ions in AIrO3 iridates, explaining J=1/2 deviations in CdIrO3, while ilmenite and hyperhoneycomb ZnIrO3 have matching local parameters so their magnetic differences arise from lattice connectivity.","pipeline_version":"pith-pipeline@v0.9.0","pith_extraction_headline":"Local multiplet parameters match in ilmenite and hyperhoneycomb ZnIrO3, showing lattice structure alone controls their distinct magnetic states.","strongest_claim":"The local multiplet parameters of ilmenite ZnIrO3 and hyperhoneycomb β-ZnIrO3 are found to be nearly identical, demonstrating that their different magnetic ground states are primarily governed by their distinct lattice structures rather than the single-ion properties.","weakest_assumption":"The multiplet model used to fit the RIXS spectra fully captures the crystal-field and intraionic parameters without significant unaccounted contributions from covalency, phonons, or other many-body effects that could alter the extracted values."}},"verdict_id":"871d16fb-ffa1-4ab5-b524-a986e6da2bf9"}}],"author_attestations":[],"timestamp_anchors":[],"storage_attestations":[],"citation_signatures":[],"replication_records":[],"corrections":[],"mirror_hints":[],"record_created":{"event_id":"sha256:04a47d89438e7b5bc77eb52b17f2809e10dcb75da0af0f8dda47531cf1cbb066","target":"record","created_at":"2026-06-10T01:10:00Z","signer":{"key_id":"pith-v1-2026-05","public_key_fingerprint":"8d4b5ee74e4693bcd1df2446408b0d54","signer_id":"pith.science","signer_type":"pith_registry"},"payload":{"attestation_state":"computed","canonical_record":{"metadata":{"abstract_canon_sha256":"bcbb291de0144af9cad492abc438be8b13baab14fc7666c1e4ede30d4e5b94e0","cross_cats_sorted":[],"license":"http://creativecommons.org/licenses/by/4.0/","primary_cat":"cond-mat.str-el","submitted_at":"2026-04-10T04:02:58Z","title_canon_sha256":"14ce42b7587001591ba671c02186c26bf7b636cb31265f899e445a73c759eb85"},"schema_version":"1.0","source":{"id":"2604.08934","kind":"arxiv","version":1}},"canonical_sha256":"035d490706f688d45e7fa8f6955a5e16f4d2c24d3c24a46b44494b64fe757659","receipt":{"algorithm":"ed25519","builder_version":"pith-number-builder-2026-05-17-v1","canonical_sha256":"035d490706f688d45e7fa8f6955a5e16f4d2c24d3c24a46b44494b64fe757659","first_computed_at":"2026-06-10T01:10:00.513817Z","key_id":"pith-v1-2026-05","kind":"pith_receipt","last_reissued_at":"2026-06-10T01:10:00.513817Z","public_key_fingerprint":"8d4b5ee74e4693bcd1df2446408b0d54","receipt_version":"0.3","signature_b64":"5Moe85xmiRvj6WENwq57GacXE+cKgNLYGNlkCowqQ5lljyoGVvqESbwjXvCGb+pN9PZhUL6iQt2/2fClOCMZDA==","signature_status":"signed_v1","signed_at":"2026-06-10T01:10:00.514867Z","signed_message":"canonical_sha256_bytes"},"source_id":"2604.08934","source_kind":"arxiv","source_version":1}}},"equivocations":[],"invalid_events":[],"applied_event_ids":["sha256:04a47d89438e7b5bc77eb52b17f2809e10dcb75da0af0f8dda47531cf1cbb066","sha256:b0e33e89a55692587f6964a8cf407942e0c19f5f302489f7f563007540ee2c5b"],"state_sha256":"0643353ea4f0c2755b9422d3fb8a33b574da15e2cd4323d1d4e6f11725c8bd63"}