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arxiv 1703.04707 v1 pith:DC5DG4CO submitted 2017-03-14 cond-mat.mes-hall cond-mat.mtrl-sciquant-ph

Controlled dynamic screening of excitonic complexes in 2D semiconductors

classification cond-mat.mes-hall cond-mat.mtrl-sciquant-ph
keywords dynamicmodelscreeningexcitonexcitonicexcitonsscreenedagreement
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We report a combined theoretical/experimental study of dynamic screening of excitons in media with frequency-dependent dielectric functions. We develop an analytical model showing that interparticle interactions in an exciton are screened in the range of frequencies from zero to the characteristic binding energy depending on the symmetries and transition energies of that exciton. The problem of the dynamic screening is then reduced to simply solving the Schrodinger equation with an effectively frequency-independent potential. Quantitative predictions of the model are experimentally verified using a test system: neutral, charged and defect-bound excitons in two-dimensional monolayer WS2, screened by metallic, liquid, and semiconducting environments. The screening-induced shifts of the excitonic peaks in photoluminescence spectra are in good agreement with our model.

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