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arxiv 2303.00419 v1 pith:XFO546XV submitted 2023-03-01 cond-mat.mes-hall cond-mat.mtrl-scicond-mat.quant-gas

Electrical control of hybrid exciton transport in a van der Waals heterostructure

classification cond-mat.mes-hall cond-mat.mtrl-scicond-mat.quant-gas
keywords excitontransportexcitonscontroldegreesgasesheterostructurehybridization
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has hitherto limited the degrees of tunability and the microscopic understanding of exciton transport. In this work, we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with dominating radiative decay mechanisms over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases and have crucial implications for the study of emerging states of matter, such as Bose-Einstein condensation, as well as for optoelectronic applications based on exciton propagation.

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  1. Unveiling the Spin-Valley Structure of Dipolar Exciton Ladders in R-stacked WSe$_2$/WS$_2$ Moir\'e Heterobilayers

    cond-mat.mes-hall 2026-07 conditional novelty 6.0

    Helicity-resolved magneto-photoluminescence reveals that the unequal spacing of the dipolar exciton ladder in R-stacked WSe₂/WS₂ arises from triplet and singlet spin-valley two-exciton states, not simple occupation-nu...