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Coupled magnetic and electric hysteresis in the multiferroic double perovskite Lu2MnCoO6

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arxiv 1409.5072 v2 pith:N4A5L4BZ submitted 2014-09-17 cond-mat.mtrl-sci

Vivien S. Zapf , B. G. Ueland , Mark Laver , Martin Lonsky , Merlin Pohlit , Jens Müller , Tom Lancaster , Johannes S. Möller
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Stephen J. Blundell John Singleton Jorge Mira Susana Yañez-Vilar Maria Antonia Señarís-Rodríguez
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classification cond-mat.mtrl-sci
keywords hysteresismagneticcoupledelectrichystereticlu2mncoo6multiferroicspin
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We investigate a magnetic hysteresis loop with a remanent moment that couples to electric polarization to create coupled hysteretic multiferroic behavior in Lu2MnCoO6. Measurements of elastic neutron diffraction, muon spin relaxation, and micro-Hall magnetometry demonstrate an unusual mechanism for the magnetic hysteresis, namely the hysteretic evolution of a microscopic magnetic order, and not classic ferromagnetic domain effects. We show how the frustrated spin system evolves from antiferromagnetism with an incommensurate long-wavelength modulation and strong fluctuations towards a net magnetism. We also clarify the different temperature scales for the onset of ordering, dynamics, and hysteresis.

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  1. Exploring magneto-electric coupling through lattice distortions: insights from a pantograph model

    cond-mat.str-el 2025-05 conditional novelty 2.0 of 10

    The pantograph model, reviewed from the authors' prior works, shows that lattice-distortion-mediated coupling between spins and dipoles can produce polarization switch-off and magnetization plateaus in type II colline...

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