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Emergent spin-charge-orbital order in superconductor La$_3$Ni$_2$O$_7$

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arxiv 2407.18473 v1 pith:ZRVPZY55 submitted 2024-07-26 cond-mat.supr-con

classification cond-mat.supr-con
keywords orderemphmagneticsuperconductivitychargedensityexhibitsmechanism
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abstract

The bilayer nickelate La$_3$Ni$_2$O$_7$ (LNO) exhibits a remarkably high-temperature superconductivity of approximately 80 K under pressure, sparking considerable attentions. However, the nature of the spin, charge, and orbital order in LNO remains unknown, hindering the exploration of the mechanism of superconductivity. Here, supported by symmetry analysis and density functional theory calculations, we unravel a double strip ground state of LNO with alternating magnetic moments arrangements. Interestingly, a charge density wave emerges under this determined magnetic order. Such CDW phase exhibits a Pmnm space group with breathing deformation of the NiO$_6$ octahedra, where the stretching and shrinking of the octahedra correspond to the formation of \emph{d}$_{z^2}^1$\emph{d}$_{x^2-y^2}^1$ and \emph{d}$_{z^2}^1$ orbital order. Moreover, we build a first-principles-based Hamiltonian for LNO, which provides deeper insight into its peculiar magnetic order. Our work thus reveals a systematic spin-charge-orbital picture for LNO, which can be extended to other nickelate-based superconductors, paving the way for determining the mechanism of superconductivity.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Origin of the Diagonal Double-Stripe Spin-Density-Wave and Potential Superconductivity in Bulk La$_3$Ni$_2$O$_{7}$ at Ambient Pressure

    cond-mat.supr-con 2024-12 conditional novelty 6.0 of 10

    An RPA analysis of an eight-band tight-binding model for ambient-pressure La3Ni2O7 reproduces the experimentally observed unidirectional diagonal double-stripe spin-density-wave and predicts enhanced pairing under hol...

  2. Spin density wave and superconductivity in the bilayer $t$-$J$ model of $\rm{La}_{3}Ni_{2}O_{7}$ under renormalized mean-field theory

    cond-mat.supr-con 2024-12 conditional novelty 5.0 of 10

    A renormalized mean-field study of a bilayer t-J model predicts antiferromagnetic d-wave and double-spin-stripe s-wave coexistence states in La3Ni2O7, with the transition tuned by inter-layer coupling.

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