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Layer-dependent field-free switching of N\'eel vector in a van der Waals antiferromagnet

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arxiv 2504.06764 v1 pith:SUPKQP56 submitted 2025-04-09 cond-mat.mes-hall

classification cond-mat.mes-hall
keywords antiferromagneticfcgtspinswitchingvectorantiferromagnetantiferromagnetselectrical
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abstract

Two-dimensional antiferromagnets, combining the dual advantages of van der Waals (vdW) and antiferromagnetic materials, provide an unprecedented platform for exploring emergent spin-related phenomena. However, electrical manipulation of N\'eel vectors in vdW antiferromagnets - the cornerstone of antiferromagnetic spintronics - remains challenging. Here, we report layer-dependent electrical switching of the N\'eel vector in an A-type vdW antiferromagnet $(Fe,Co)_3$$GaTe_2$ (FCGT) with perpendicular magnetic anisotropy. The N\'eel vector of FCGT with odd-number vdW layers can be 180{\deg} reversed via spin-orbit torques. Furthermore, we achieve field-free switching in an all-vdW, all-antiferromagnet heterostructure of FCGT/CrSBr in which the noncollinear interfacial spin texture breaks the mirror symmetry. Our results establish layer-controlled spin symmetries and interfacial spin engineering as universal paradigms for manipulating antiferromagnetic order, paving the way for realising reliable and efficient vdW antiferromagnetic devices.

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  1. Interface-controlled antiferromagnetic tunnel junctions

    cond-mat.mtrl-sci 2025-06 conditional novelty 6.0 of 10

    A-type antiferromagnetic electrodes with uncompensated interfaces can generate a large negative tunneling magnetoresistance, computed here at about -300 percent in Fe4GeTe2 junctions.

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