Vibrationally mediated Dzyaloshinskii-Moriya interaction from torsional modes explains high spin selectivity in photo-excited chiral donor-acceptor molecules.
In this case, in order to keep the overall transfer rate equal, the system-bath coupling operator is given by ˆXD = cosθ X σ c† 1σcDσ +isinθ X σ,σ′ c† 1σσz σσ ′cDσ′ (S13) 12
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Vibrationally-mediated Dzyaloshinskii-Moriya interaction as the origin of Chirality-Induced Spin Selectivity in donor-acceptor molecules
Vibrationally mediated Dzyaloshinskii-Moriya interaction from torsional modes explains high spin selectivity in photo-excited chiral donor-acceptor molecules.