A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.
P.et al.Few-femtosecond soft x-ray transient absorption spectroscopy with tuneable DUV-Vis pump pulses.Optica11, 1320–1323 (2024)
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Molecular Attoscope: Pulse Shape Spectroscopy of Electronic Coherence
A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.