Plasmon-exciton coupling in Au nanostructures with J-aggregates produces a 30 meV Rabi splitting and reduces mode lifetimes from 50 fs to 10 fs mainly through dissipation into dark states.
1-6 Polaritons arise when the rate of energy exchange between a photonic mode and an optical transition of a semiconductor or molecular system exceeds their respective decay rates
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Plasmon-Exciton Coupling and Dephasing in Hybrid Au Nanostructure/J-Aggregate Systems
Plasmon-exciton coupling in Au nanostructures with J-aggregates produces a 30 meV Rabi splitting and reduces mode lifetimes from 50 fs to 10 fs mainly through dissipation into dark states.