A bath-engineering quantum simulation framework enables numerically exact 2D spectroscopy calculations for open quantum systems, demonstrated on a driven four-level system and on Rh(CO)2C5H7O2 in chloroform where it reproduces key experimental spectral features.
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Numerical simulations demonstrate that varying excitation-pulse intensity controls coherent pathway contributions and enables selective on/off switching of spectral features in 2D spectra of a V-type system.
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Numerically-Exact Quantum-Simulation Approach for Two-Dimensional Spectroscopy of Open Quantum Systems
A bath-engineering quantum simulation framework enables numerically exact 2D spectroscopy calculations for open quantum systems, demonstrated on a driven four-level system and on Rh(CO)2C5H7O2 in chloroform where it reproduces key experimental spectral features.
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Excitation-pulse intensity mediated control of coherent nonlinear optical response of a V-type system
Numerical simulations demonstrate that varying excitation-pulse intensity controls coherent pathway contributions and enables selective on/off switching of spectral features in 2D spectra of a V-type system.