A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.
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N-mode quantized anharmonic vibronic Hamiltonians provide a second-quantized framework for DMRG-based quantum dynamics, demonstrated via excited-state simulations of maleimide.
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Molecular Attoscope: Pulse Shape Spectroscopy of Electronic Coherence
A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.
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N-Mode Quantized Anharmonic Vibronic Hamiltonians for Matrix Product State Dynamics
N-mode quantized anharmonic vibronic Hamiltonians provide a second-quantized framework for DMRG-based quantum dynamics, demonstrated via excited-state simulations of maleimide.