Grafting flexible side chains onto MOFs triggers a crossover to glass-like thermal transport by turning acoustic phonons into critically damped modes via resonant hybridization and steric crowding.
Homogeneous nonequilibrium molecular dy- namics method for heat transport and spectral decom- position with many-body potentials
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Structurally Triggered Breakdown of the Phonon Gas Model in Crystalline Metal-Organic Frameworks
Grafting flexible side chains onto MOFs triggers a crossover to glass-like thermal transport by turning acoustic phonons into critically damped modes via resonant hybridization and steric crowding.