Non-equilibrium dark excitons in homobilayer 2H-MoS2 form in 85 fs and thermalize in 150 fs, directly fingerprinted by momentum-resolved photoemission spectral function and matched by microscopic calculations.
Since the incident angle of the s-polarized pump photons in 22◦, following Fresnel equations, 26.3% percent of the incident fluence is transmitted into the sample
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The role of non-equilibrium populations in dark exciton formation
Non-equilibrium dark excitons in homobilayer 2H-MoS2 form in 85 fs and thermalize in 150 fs, directly fingerprinted by momentum-resolved photoemission spectral function and matched by microscopic calculations.