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arxiv: 1702.02476 · v1 · pith:NW2D7ULSnew · submitted 2017-02-08 · 🪐 quant-ph · physics.atom-ph

Nonlinear effects in photoionization over a broad photon-energy range within the TDCIS scheme

classification 🪐 quant-ph physics.atom-ph
keywords ionizationnonlinearrangeabove-thresholdbroadphoton-energyregimeresonance
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The present tutorial provides an overview of the time-dependent configuration interaction singles (\acs{TDCIS}) scheme applied to nonlinear ionization over a broad photon-energy range. The efficient propagation of the wave function and the calculation of photoelectron spectra within this approach are described and demonstrated in various applications. Above-threshold ionization of argon and xenon in the extreme ultraviolet energy range is investigated as an example. A particular focus is put on the xenon $4d$ giant dipole resonance and the information that nonlinear ionization can provide about resonance substructure. Furthermore, above-threshold ionization is studied in the x-ray regime and the intensity regime, at which multiphoton ionization starts to play a role at hard x-ray photon energies, is identified.

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