Strictly Non-Adiabatic Quantum Control of the Acetylene Dication Using an Infrared Field
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classification
physics.chem-ph
quant-ph
keywords
controlnon-adiabaticacetylenedicationpathwaystrictlyaffectaround
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We demonstrate the existence of a strictly non-adiabatic control pathway in deprotonation of the acetylene dication. This pathway is identified experimentally by measuring a kinetic energy shift in an ion coincidence experiment. We use a TDSE simulation to identify which properties most strongly affect our control. We find that resonant control around conical intersections is limited by the speed of non-adiabatic dynamics.
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