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Correlated insulator of excitons in WSe2/WS2 moir\'e superlattices

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arxiv 2207.10764 v2 pith:WDXXODD3 submitted 2022-07-21 cond-mat.str-el cond-mat.mes-hall

classification cond-mat.str-elcond-mat.mes-hall
keywords correlatedinsulatorbosonicmoirsuperlatticeschargeexcitonsengineering
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A panoply of unconventional electronic states has been observed in moir\'e superlattices. Engineering similar bosonic phases remains, however, largely unexplored. We report the observation of a bosonic correlated insulator in WSe2/WS2 moir\'e superlattices composed of excitons, i.e., tightly bound electron-hole pairs. We develop a pump probe spectroscopy method that we use to observe an exciton incompressible state at exciton filling {\nu}_ex = 1 and charge neutrality, indicating a correlated insulator of excitons. With varying charge density, the bosonic correlated insulator continuously transitions into an electron correlated insulator at charge filling {\nu}_e = 1, suggesting a mixed correlated insulating state between the two limits. Our studies establish semiconducting moir\'e superlattices as an intriguing platform for engineering bosonic phases.

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  1. Unveiling the Spin-Valley Structure of Dipolar Exciton Ladders in R-stacked WSe$_2$/WS$_2$ Moir\'e Heterobilayers

    cond-mat.mes-hall 2026-07 conditional novelty 6.0 of 10

    Helicity-resolved magneto-photoluminescence reveals that the unequal spacing of the dipolar exciton ladder in R-stacked WSe₂/WS₂ arises from triplet and singlet spin-valley two-exciton states, not simple occupation-nu...

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