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arxiv 2307.14693 v1 pith:YLGVZNVL submitted 2023-07-27 cond-mat.mtrl-sci physics.optics

High-harmonic spectroscopy of strongly bound excitons in solids

classification cond-mat.mtrl-sci physics.optics
keywords excitonsexcitonhigh-harmonicdemonstratepopulationsignaturessimulationsspectra
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We explore the nonlinear response of ultrafast strong-field driven excitons in a one-dimensional solid with ab initio simulations. We demonstrate from our simulations and analytical model that a finite population of excitons imprints unique signatures to the high-harmonic spectra of materials. We show the exciton population can be retrieved from the spectra. We further demonstrate signatures of exciton recombination and that a shift of the exciton level is imprinted into the harmonic signal. The results open the door to high-harmonic spectroscopy of excitons in condensed-matter systems.

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