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arxiv: 2410.18134 · v2 · pith:PNRH5ED5 · submitted 2024-10-21 · physics.ins-det · nucl-ex

A method to detect the VUV photons from cooled ²²⁹Th:CaF₂ crystals

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classification physics.ins-det nucl-ex
keywords crystalsnuclearcoolingcrystalclockscopperdamagedetection
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Thorium-229, with its exceptionally low-energy nuclear excited state, is a key candidate for developing nuclear clocks. $^{229}$Th-doped CaF$_2$ crystals, benefiting from calcium fluoride's wide band gap, show great promise as solid-state nuclear clock materials. These crystals are excited by vacuum ultraviolet (VUV) lasers, which over time cause radiation damage. Cooling the crystals can mitigate this damage but introduces a challenge: photoabsorption. This occurs when residual gas molecules condense on the crystal surface, absorbing VUV photons and deteriorating detection efficiency. To solve this, we developed a cooling technique using a copper shield to surround the crystal, acting as a cold trap. This prevents ice-layer formation, even at temperatures below $-100\,^\circ$C, preserving high VUV photon detection efficiency. Our study detailed the experimental cooling setup and demonstrated the effectiveness of the copper shield in maintaining crystal performance, a critical improvement for future solid-state nuclear clocks operating at cryogenic temperatures.

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