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Designing spin and orbital exchange Hamiltonians with ultrashort electric field transients

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arxiv 1703.03269 v1 pith:EGKWXHL5 submitted 2017-03-09 cond-mat.str-el

classification cond-mat.str-el
keywords exchangehamiltoniansorbitalspintime-dependentarbitrarycontrolelectric
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We demonstrate how electric fields with arbitrary time profile can be used to control the time-dependent parameters of spin and orbital exchange Hamiltonians. Analytic expressions for the exchange constants are derived from a time-dependent Schrieffer-Wolff transformation, and the validity of the resulting effective Hamiltonian is verified for the case of a quarter-filled two-orbital Hubbard model, by comparing to the results of a full nonequilibrium dynamical mean-field theory simulation. The ability to manipulate Hamiltonians with arbitrary time-dependent fields, beyond the paradigm of Floquet engineering, opens the possibility to control intertwined spin and orbital order using laser or THz pulses which are tailored to minimize electronic excitations.

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Cited by 2 Pith papers

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  1. $\eta$--paired superconducting hidden phase in photodoped Mott insulators

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    Photodoping a repulsive Hubbard Mott insulator can stabilize a metastable eta-pairing superconducting phase, detectable through a zero-frequency conductivity peak and negative high-frequency conductivity.

  2. Nonthermal order by disorder

    cond-mat.str-el 2024-12 conditional novelty 6.0 of 10

    Anisotropic, nonthermal fluctuations can transiently stabilize order parameter configurations that are not minima of the equilibrium free energy, through mutual feedback between order and fluctuations.

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