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Magnons, Phonons, and Thermal Hall Effect in Candidate Kitaev Magnet $\alpha$-RuCl$_3$

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arxiv 2301.07401 v2 pith:DTNCPNUQ submitted 2023-01-18 cond-mat.str-el

classification cond-mat.str-el
keywords hallthermalalphaeffectkappaphononsruclintrinsic
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abstract

We study the nature of the debated thermal Hall effect in the candidate Kitaev material $\alpha$-RuCl$_3$. Without assuming the existence of a gapped spin liquid, we show that a realistic minimal spin model in the canted zigzag phase suffices, at the level of linear spin-wave theory, to qualitatively explain the observed temperature and magnetic field dependence of the non-quantized thermal Hall conductivity $\kappa_{xy}$, with its origin lying in the Berry curvature of the magnon bands. The magnitude of the effect is however too small compared to the measurement by Czajka et al. [Nat. Mater. 22, 36-41 (2023)], even after scanning a broad range of model parameters so as to maximize $\kappa_{xy}/T$. Recent experiments suggest that phonons play an important role, which we show couple to the spins, endowing phonons with chirality. The resulting intrinsic contribution, from both magnons and phonons, is however still insufficient to explain the observed magnitude of the Hall signal. After careful analysis of the extrinsic phonon mechanisms, we use the recent experimental data on thermal transport in $\alpha$-RuCl$_3$ by Lefran\c{c}ois et al. [Phys. Rev. X 12, 021025 (2022)] to determine the phenomenological ratio of the extrinsic and intrinsic contributions $\eta\equiv \kappa_{xy}^{E}/\kappa_{xy}^{I}$. We find $\eta=1.2\pm 0.5$, which when combined with our computed intrinsic value, explains quantitavely both the magnitude and detailed temperature dependence of the experimental thermal Hall effect in $\alpha$-RuCl$_3$.

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  1. The Saga of $\alpha$-RuCl$_3$: Parameters, Models, and Phase Diagrams

    cond-mat.str-el 2025-02 conditional novelty 6.0 of 10

    Using the tilt angle, high-field ESR gap, and critical-field difference, the authors constrain the anisotropic exchanges of the effective spin model of alpha-RuCl3 and identify two counter-rotating helical phases near...

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