Pith. sign in

REVIEW 1 cited by

Anomalous amplitude mode dynamics below the expected charge-density-wave transition in 1$T$-VSe$_2$

Not yet reviewed by Pith; the record is open.

This paper has not been read by Pith yet. Machine review is queued; the pith claim, tier, and objections will appear here once it completes.

SPECIMEN: schema-true, not a live event

T0 review · schema-true

One-sentence machine reading of the paper's core claim.

pith:XXXXXXXX · record.json · timestamp

arxiv 2408.16510 v1 pith:R6ABXZPJ submitted 2024-08-29 cond-mat.str-el

classification cond-mat.str-el
keywords amplitudeelectroniclatticemodeorderphasetemperaturetransition
verification ladder T0 review T1 audit T2 compute T3 formal

Signed reviews

No signed human review yet.

0 comments
abstract

A charge-density-wave (CDW) is characterized by a dynamical order parameter consisting of a time-dependent amplitude and phase, which manifest as optically-active collective modes of the CDW phase. Studying the behaviour of such collective modes in the time-domain, and their coupling with electronic and lattice order, provides important insight into the underlying mechanisms behind CDW formation. In this work, we report on femtosecond broadband transient reflectivity experiments on bulk 1$T$-VSe$_2$ using near-infrared excitation. At low temperature, we observe coherent oscillations associated with the CDW amplitude mode and phonons of the distorted lattice. Across the expected transition temperature at 110 K, we confirm signatures of a rearrangement of the electronic structure evident in the quasiparticle dynamics. However, we find that the amplitude mode instead softens to zero frequency at 80 K, possibly indicating an additional phase transition at this temperature. In addition, we demonstrate photoinduced CDW melting, associated with a collapse of the electronic and lattice order, which occurs at moderate excitation densities, consistent with a dominant electron-phonon CDW mechanism.

Discussion (0). Continue with ORCID to comment.

Forward citations

Cited by 1 Pith paper

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Time-domain decoding of unconventional charge order mechanisms in nonmagnetic and magnetic kagome metals

    cond-mat.str-el 2025-06 conditional novelty 7.0 of 10

    Charge order in kagome metal FeGe is resilient to ultrafast photoexcitation, unlike ScV6Sn6, indicating a magnetism-interlocked order with a triple-well free energy landscape.

Pith tools