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Striped magnetization plateau and chirality-reversible anomalous Hall effect in a magnetic kagome metal
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abstract
Kagome materials with magnetic frustration in two-dimensional networks are known for their exotic properties, such as the anomalous Hall effect (AHE) with non-collinear spin textures. However, the effects of one-dimensional (1D) spin chains within these networks are less understood. Here, we report a distinctive AHE in the bilayer-distorted kagome material GdTi$_3$Bi$_4$, featuring 1D Gd zigzag spin chains, a one-third magnetization plateau, and two successive metamagnetic transitions. At these metamagnetic transitions, Hall resistivity shows abrupt jumps linked to the formation of stripe domain walls, while within the plateau, the absence of detectable domain walls suggests possible presence of skyrmion phase. Reducing the sample size to a few microns reveals additional Hall resistivity spikes, indicating domain wall skew scattering contributions. Magnetic atomistic spin dynamics simulations reveal that the magnetic textures at these transitions have reverse chirality, explaining the evolution of AHE and domain walls with fields. These results underscore the potential of magnetic and crystal symmetry interplay, and magnetic field-engineered spin chirality, for controlling domain walls and tuning transverse properties, advancing spintronic applications.
Forward citations
Cited by 2 Pith papers
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Spin density wave and van Hove singularity in the kagome metal CeTi3Bi4
CeTi3Bi4 exhibits an incommensurate spin density wave of cerium moments coexisting with commensurate antiferromagnetism, with wave vectors matching van Hove singularities near the Fermi level.
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Synergistic doping and stabilization of magnetically tunable LnTi$_3$(Sb,Sn)$_4$ (Ln:Ce--Gd) kagome metals
In LnTi3(Sb,Sn)4 kagome metals, Sb/Sn alloying stabilizes a structure with no pure endpoints and tunes the Sm series between AFM, FM, and mixed A(FM) magnetic states.
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