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Interplay of Charge Density Wave and Magnetism on the Kagom\'e Lattice

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arxiv 2409.03063 v2 pith:YG5G53JJ submitted 2024-09-04 cond-mat.str-el

classification cond-mat.str-el
keywords kagombond-orderedlatticechargedensityhovemagneticonsite
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abstract

Motivated by the recent discovery of charge density wave (CDW) order in the magnetic kagom\'e metal FeGe, we study the single-orbital $t$-$U$-$V_1$-$V_2$ model on the kagom\'e lattice, where $U$, $V_1$, and $V_2$ are the onsite, nearest neighbor, and next-nearest-neighbor Coulomb repulsions, respectively. When the Fermi level lies in the flat band, the instability toward ferromagnetic (FM) order gives rise to a FM half-metal at sufficiently large onsite $U$. Intriguingly, at band filling $n=17/24$, the Fermi level crosses the van Hove singularity of the spin-minority bands of the half-metal. We show that, due to the unique geometry and sublattice interference on the kagom\'e lattice at van Hove singularity, the intersite Coulomb interactions $V_1$ and $V_2$ drive a real and an imaginary bond-ordered $2a_0 \times 2a_0$ CDW instability, respectively. The FM loop current CDW with complex bond orders is a spin-polarized Chern insulator exhibiting the quantum anomalous Hall effect. The bond fluctuations are found to be substantially enhanced compared to the corresponding nonmagnetic kagom\'e metals at van Hove filling, providing a concrete model realization of the bond-ordered CDWs, including the FM loop current CDW, over the onsite charge density ordered states. When the spins are partially polarized, we find that the formation of bond-ordered CDWs enhances substantially the ordered magnetic moments. These findings provide physical insights for the emergence of loop-current and bond-ordered CDW and their interplay with magnetism on the kagom\'e lattice, with possible connections to the magnetic kagom\'e metal FeGe.

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  1. Ultrafast optical control of charge orders in kagome metals

    cond-mat.str-el 2024-11 conditional novelty 6.0 of 10

    Time-dependent Hartree-Fock simulations predict that linearly polarized pump pulses create directional and nematic charge-order responses in kagome metals, while circularly polarized pulses induce loop-current charge order.

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