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arxiv: 2605.09172 · v1 · submitted 2026-05-09 · ❄️ cond-mat.soft · physics.flu-dyn

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Lubrication-Induced Newtonianization Enables Passive Transport of Non-Newtonian materials

Arvind Arun Dev, Bernard Doudin, Paszkal Papp, Thomas M. Hermans

Authors on Pith no claims yet

Pith reviewed 2026-05-12 01:50 UTC · model grok-4.3

classification ❄️ cond-mat.soft physics.flu-dyn
keywords lubricationnon-Newtonian fluidsshear localizationNewtonianizationpassive transportboundary layeryield-stress materialscomplex fluids
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The pith

Stable boundary lubrication localizes shear in a thin layer, making non-Newtonian materials flow as if they were Newtonian fluids governed by geometry and the lubricant rather than their bulk properties.

A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.

The paper shows that a thin, stable lubricating layer at the walls of a conduit can suppress the nonlinear flow behavior typical of complex fluids. Yield-stress fluids, shear-thinning materials, and thixotropic substances normally demand high pressure gradients to move through narrow spaces because their viscosity or yield point changes with rate. When shear is forced into the low-viscosity boundary layer, the overall transport rate becomes set by the layer thickness, the channel geometry, and the lubricant viscosity instead. This decoupling allows the same materials to be driven at far lower forces, including passive gravity-driven flow that produces much higher throughput than occurs in rigid-wall channels. The result holds across analytical solutions of Stokes flow and numerical simulations for a broad class of non-Newtonian fluids.

Core claim

Lubrication-induced shear localization leads to an apparent Newtonianization of transport, in which the macroscopic flow response becomes primarily controlled by the lubricating layer and geometric confinement rather than the intrinsic material properties. Materials that would otherwise require large pressure gradients can be transported at substantially lower driving forces, and boundary-dominated transport enables gravity-driven passive flow with orders-of-magnitude enhancement in throughput compared to rigid-wall conduits.

What carries the argument

Lubrication-induced shear localization within a thin, low-viscosity interfacial boundary layer that decouples bulk rheology from macroscopic flow.

If this is right

  • Yield-stress, shear-dependent, and thixotropic materials flow at rates set by lubricant properties and confinement geometry instead of their own nonlinear rheology.
  • Transport becomes possible at driving forces far below those predicted by bulk rheology alone.
  • Gravity alone can drive passive flow with throughput increased by orders of magnitude relative to rigid conduits.
  • The effect applies across a broad class of complex fluids provided a stable boundary layer forms.

Where Pith is reading between the lines

These are editorial extensions of the paper, not claims the author makes directly.

  • Designs for energy-efficient pumping or gravity-fed transport of pastes, gels, and slurries could exploit thin lubricant films to bypass bulk rheology limits.
  • Biological conduits that naturally maintain lubricating layers, such as certain ducts or vascular segments, may achieve similar simplifications in material transport.
  • Varying lubricant viscosity or layer thickness offers a tunable control parameter for flow rate without changing the transported material itself.
  • The same localization principle might be tested in oscillatory or time-varying flows to check whether thixotropic recovery is also suppressed.

Load-bearing premise

A thin, low-viscosity lubrication layer remains stable and intact under flow without mixing into the bulk or losing its low-viscosity character for many different non-Newtonian materials.

What would settle it

Direct measurement of the velocity profile across the channel that shows significant shear occurring inside the bulk material rather than being confined to a thin boundary layer, or observation that the required driving pressure still scales with the bulk yield stress or viscosity even when lubricant is present.

read the original abstract

Non Newtonian flows are typically governed by intrinsic bulk rheology, which imposes strong constraints on transport through confined geometries. Here, we show that stable boundary lubrication can fundamentally alter this behavior by localizing shear within a thin, low-viscosity interfacial layer. As a result, the nonlinear rheological response of a broad class of complex materials, including yield-stress, shear-dependent, and thixotropic materials, is strongly suppressed during flow. Using analytical solutions of Stokes flow and numerical simulations, we demonstrate that lubrication-induced shear localization leads to an apparent Newtonianization of transport, in which the macroscopic flow response becomes primarily controlled by the lubricating layer and geometric confinement rather than the intrinsic material properties. In this regime, materials that would otherwise require large pressure gradients can be transported at substantially lower driving forces. Notably, this boundary-dominated transport enables gravity-driven passive flow with orders-of-magnitude enhancement in throughput compared to rigid-wall conduits. These results establish lubrication as a powerful mechanism for tuning and simplifying complex fluid transport, with implications for biological systems, soft and jammed materials, and energy-efficient fluids.

Editorial analysis

A structured set of objections, weighed in public.

Desk editor's note, referee report, simulated authors' rebuttal, and a circularity audit. Tearing a paper down is the easy half of reading it; the pith above is the substance, this is the friction.

Referee Report

2 major / 2 minor

Summary. The manuscript claims that stable boundary lubrication in confined geometries localizes shear within a thin, low-viscosity interfacial layer for a broad class of non-Newtonian materials (yield-stress, shear-dependent, and thixotropic). This suppresses intrinsic nonlinear rheology, producing apparent Newtonianization of macroscopic transport as shown by analytical Stokes-flow solutions and numerical simulations. The result enables passive gravity-driven flow with orders-of-magnitude throughput enhancement relative to rigid-wall conduits.

Significance. If the lubrication layer remains stable and emergent, the work identifies a mechanism to decouple transport from bulk nonlinearities, with clear implications for energy-efficient handling of complex fluids in biological, soft-matter, and industrial contexts. The use of both analytical Stokes solutions and simulations is a methodological strength that allows direct comparison of lubrication-dominated versus bulk-dominated regimes.

major comments (2)
  1. [Numerical Simulations] The central claim that nonlinear bulk responses are bypassed rests on the persistence of a thin, low-viscosity boundary layer that localizes all shear. In the numerical simulations section, the layer thickness and viscosity contrast appear to be imposed as boundary conditions rather than emerging self-consistently from the non-Newtonian constitutive model (yield stress, thixotropy, or particle migration). Because the Stokes equations are linear, this imposition does not automatically guarantee layer stability under flow for materials that can yield or restructure; a derivation or simulation showing the layer as an output (e.g., via coupled interface evolution) is required for the “apparent Newtonianization” to hold across the claimed material class.
  2. [Analytical Stokes Solutions] § on analytical Stokes solutions: the closed-form solutions assume a fixed two-layer geometry with a prescribed low-viscosity film. While this yields linear pressure-flow relations, it does not address whether the film thickness remains constant or migrates when the bulk is allowed to yield or exhibit thixotropy; without a stability analysis or time-dependent simulation of the interface, the extrapolation to passive gravity-driven transport remains conditional on the layer assumption.
minor comments (2)
  1. Figure captions should explicitly state the constitutive model parameters (e.g., yield stress, thixotropic time scale) and the imposed lubrication-layer viscosity ratio used in each panel to allow direct comparison with the analytical results.
  2. The abstract states “orders-of-magnitude enhancement”; the corresponding figure or table should report the exact throughput ratios and the range of Bond numbers or pressure gradients over which the enhancement is observed.

Simulated Author's Rebuttal

2 responses · 0 unresolved

We thank the referee for their careful reading and constructive comments, which help clarify the scope and assumptions of our work on lubrication-induced Newtonianization. We respond to each major comment below and outline the corresponding revisions.

read point-by-point responses
  1. Referee: [Numerical Simulations] The central claim that nonlinear bulk responses are bypassed rests on the persistence of a thin, low-viscosity boundary layer that localizes all shear. In the numerical simulations section, the layer thickness and viscosity contrast appear to be imposed as boundary conditions rather than emerging self-consistently from the non-Newtonian constitutive model (yield stress, thixotropy, or particle migration). Because the Stokes equations are linear, this imposition does not automatically guarantee layer stability under flow for materials that can yield or restructure; a derivation or simulation showing the layer as an output (e.g., via coupled interface evolution) is required for the “apparent Newtonianization” to hold across the claimed material class.

    Authors: We acknowledge that the numerical simulations prescribe a fixed low-viscosity layer thickness and viscosity contrast as boundary conditions. This modeling choice isolates the macroscopic consequences of shear localization for the broad class of materials considered, under the assumption of stable boundary lubrication motivated by experimental observations. We agree that a fully self-consistent treatment in which the layer emerges from the constitutive model (e.g., via particle migration or thixotropic restructuring) would provide additional support. In the revised manuscript we will add a new subsection in the discussion that (i) reviews physical mechanisms known to produce stable lubricating layers in yield-stress and thixotropic fluids, (ii) cites relevant literature on interfacial dynamics, and (iii) explicitly states that the reported Newtonianization holds conditional on layer persistence. We will also note the value of future coupled interface-evolution simulations. revision: partial

  2. Referee: [Analytical Stokes Solutions] § on analytical Stokes solutions: the closed-form solutions assume a fixed two-layer geometry with a prescribed low-viscosity film. While this yields linear pressure-flow relations, it does not address whether the film thickness remains constant or migrates when the bulk is allowed to yield or exhibit thixotropy; without a stability analysis or time-dependent simulation of the interface, the extrapolation to passive gravity-driven transport remains conditional on the layer assumption.

    Authors: The closed-form Stokes solutions are derived for a fixed two-layer geometry to obtain exact linear pressure-flow relations that highlight the dominant role of the interfacial layer. We recognize that this idealization does not include an explicit stability analysis of the interface under yielding or thixotropy. In the revised manuscript we will expand the analytical section to include a short discussion of interface stability based on lubrication-theory scaling arguments and will qualify the passive-transport predictions as conditional on the maintenance of the low-viscosity film. These additions will be cross-referenced with the numerical results and the new discussion subsection on layer formation. revision: partial

Circularity Check

0 steps flagged

No significant circularity in derivation chain

full rationale

The paper's central demonstration relies on analytical solutions of Stokes flow and numerical simulations applied to a model incorporating a thin low-viscosity boundary lubrication layer. The resulting apparent Newtonianization of macroscopic transport follows directly as a consequence of shear localization within that layer, which is an explicit modeling choice rather than a fitted parameter or self-referential definition. No equations or claims reduce by construction to their own inputs; the suppression of bulk nonlinearities is shown as an outcome of the imposed geometry and layer properties. No load-bearing self-citations, uniqueness theorems, or ansatzes smuggled via prior work are present. This is a standard non-circular finding for a modeling study that takes the lubrication layer as a premise and derives transport implications from it.

Axiom & Free-Parameter Ledger

0 free parameters · 2 axioms · 0 invented entities

The abstract invokes standard Stokes-flow equations for slow viscous flow and assumes the existence and stability of a thin low-viscosity lubricating layer; no free parameters or new entities are explicitly introduced.

axioms (2)
  • standard math Stokes equations govern the flow
    Analytical solutions are stated to be based on Stokes flow.
  • domain assumption Stable boundary lubrication layer with low viscosity exists and persists
    Central to localizing shear away from the bulk material.

pith-pipeline@v0.9.0 · 5497 in / 1294 out tokens · 51321 ms · 2026-05-12T01:50:28.310030+00:00 · methodology

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44 extracted references · 44 canonical work pages

  1. [1]

    Kollmannsberger, B

    P. Kollmannsberger, B. Fabry, Linear and Nonlinear Rheology of Living Cells. Annu. Rev. Mater. Res. 41, 75–97 (2011)

  2. [2]

    Blaeser, D

    A. Blaeser, D. F. Duarte Campos, U. Puster, W. Richtering, M. M. Stevens, H. Fischer, Controlling Shear Stress in 3D Bioprinting is a Key Factor to Balance Printing Resolution and Stem Cell Integrity. Adv. Healthc. Mater. 5, 326–333 (2016)

  3. [3]

    P. A. Rühs, J. Bergfreund, P. Bertsch, S. J. Gstöhl, P. Fischer, Complex fluids in animal survival strategies. Soft Matter 17, 3022–3036 (2021)

  4. [4]

    Q. Jia, L. Shen, Z. Zhou, S. Wang, L. Liu, Y. Wang, Y. Li, J. Wang, Flowability, Carbon Sequestration, and Strength Properties of Carbonation-Cured Solid Waste-Based Backfilling Materials. Energy Fuels 39, 17990–18000 (2025)

  5. [5]

    J. Li, D. J. Mooney, Designing hydrogels for controlled drug delivery. Nat. Rev. Mater. 1, 16071 (2016)

  6. [6]

    https://pubchem.ncbi.nlm.nih.gov/patent /US-2006234577-A1

    Advanced body armor utilizing shear thickening fluids - Patent US-2006234577- A1 - PubChem. https://pubchem.ncbi.nlm.nih.gov/patent /US-2006234577-A1

  7. [7]

    Non- Newtonian Fluids in Environmental Engineering

    A. M. Abubakar, S. A. Wali, A. Mohammed, V. K. Pandey, “Non- Newtonian Fluids in Environmental Engineering” in Non-Newtonian Fluids for Industrial Applications (John Wiley & Sons, Ltd, 2026; https://onlinelibrary.wiley.com/doi/abs/1 0.1002/9781394356256.ch15), pp. 319– 354

  8. [8]

    J. F. Morris, Shear Thickening of Concentrated Suspensions: Recent Developments and Relation to Other Phenomena. Annu. Rev. Fluid Mech. 52, 121–144 (2020)

  9. [9]

    Cheng, J

    X. Cheng, J. H. McCoy, J. N. Israelachvili, I. Cohen, Imaging the Microscopic Structure of Shear Thinning and Thickening Colloidal Suspensions. Science 333, 1276–1279 (2011)

  10. [10]

    Pouliquen, Y

    O. Pouliquen, Y. Forterre, A non-local rheology for dense granular flows. Philos. Trans. R. Soc. Math. Phys. Eng. Sci. 367, 5091–5107 (2009)

  11. [11]

    Goyon, A

    J. Goyon, A. Colin, G. Ovarlez, A. Ajdari, L. Bocquet, Spatial Cooperativity in Soft Glassy Flows. Nature 454, 84–87 (2008)

  12. [12]

    P. Jop, V. Mansard, P. Chaudhuri, L. Bocquet, A. Colin, Microscale Rheology of a Soft Glassy Material Close to Yielding. Phys. Rev. Lett. 108, 148301 (2012)

  13. [13]

    N. J. Balmforth, I. A. Frigaard, G. Ovarlez, Yielding to Stress: Recent Developments in Viscoplastic Fluid Mechanics. Annu. Rev. Fluid Mech. 46, 121–146 (2014)

  14. [14]

    Brown, H

    E. Brown, H. M. Jaeger, Shear thickening in concentrated suspensions: phenomenology, mechanisms and relations to jamming. Rep. Prog. Phys. 77, 046602 (2014)

  15. [15]

    Brown, N

    E. Brown, N. A. Forman, C. S. Orellana, H. Zhang, B. W. Maynor, D. E. Betts, J. M. DeSimone, H. M. Jaeger, Generality of shear thickening in dense suspensions. Nat. Mater. 9, 220–224 (2010)

  16. [16]

    D. Bonn, M. M. Denn, L. Berthier, T. Divoux, S. Manneville, Yield stress materials in soft condensed matter. Rev. Mod. Phys. 89, 035005 (2017)

  17. [17]

    Coussot, Fifty shades of yield stress fluids: rheological challenges and engineering perspectives

    P. Coussot, Fifty shades of yield stress fluids: rheological challenges and engineering perspectives. Rheol. Acta 64, 167–193 (2025)

  18. [18]

    Mewis, N

    J. Mewis, N. J. Wagner, Thixotropy. Adv. Colloid Interface Sci. 147–148, 214–227 (2009)

  19. [19]

    R. G. Larson, Y. Wei, A review of thixotropy and its rheological modeling. J. Rheol. 63, 477–501 (2019)

  20. [20]

    Kayal, A

    S. Kayal, A. Q. Nguyen, D. Bi, The Rheology of Living Tissues: From Cells to Organismal Mechanics. Annu. Rev. Condens. Matter Phys. 17, 285–304 (2026)

  21. [21]

    D. A. Matoz-Fernandez, E. Agoritsas, J.-L. Barrat, E. Bertin, K. Martens, Nonlinear Rheology in a Model Biological Tissue. Phys. Rev. Lett. 118, 158105 (2017)

  22. [22]

    W. H. Herschel, R. Bulkley, Konsistenzmessungen von Gummi- Benzollösungen. Kolloid-Z. 39, 291–300 (1926)

  23. [23]

    R. P. A. Dullens, C. Bechinger, Shear Thinning and Local Melting of Colloidal Crystals. Phys. Rev. Lett. 107, 138301 (2011)

  24. [24]

    Ostwald, Ueber die Geschwindigkeitsfunktion der Viskosität disperser Systeme

    W. Ostwald, Ueber die Geschwindigkeitsfunktion der Viskosität disperser Systeme. I. Kolloid-Z. 36, 99–117 (1925)

  25. [25]

    N’gouamba, J

    E. N’gouamba, J. Goyon, L. Tocquer, T. Oerther, P. Coussot, Yielding, thixotropy, and strain stiffening of aqueous carbon black suspensions. J. Rheol. 64, 955–968 (2020)

  26. [26]

    Dullaert, J

    K. Dullaert, J. Mewis, A structural kinetics model for thixotropy. J. Non-Newton. Fluid Mech. 139, 21–30 (2006)

  27. [27]

    Zhang, Y

    L. Zhang, Y. Li, S. Zhang, X. Wang, X. Xia, D. Xie, C. Gu, J. Tu, Non-Newtonian Fluid State K–Na Alloy for a Stretchable Energy Storage Device. Small Methods 3, 1900383 (2019)

  28. [28]

    Zhang, Z

    P. Zhang, Z. W. Ma, Z. Y. Bai, J. Ye, Rheological and energy transport characteristics of a phase change material slurry. Energy 106, 63–72 (2016)

  29. [29]

    Narayanan, F

    A. Narayanan, F. Mugele, M. H. G. Duits, Mechanical History Dependence in Carbon Black Suspensions for Flow Batteries: A Rheo-Impedance Study. Langmuir 33, 1629–1638 (2017)

  30. [30]

    Duduta, B

    M. Duduta, B. Ho, V. C. Wood, P. Limthongkul, V. E. Brunini, W. C. Carter, Y.-M. Chiang, Semi-Solid Lithium Rechargeable Flow Battery. Adv. Energy Mater. 1, 511–516 (2011)

  31. [31]

    Zheng, H

    Z. Zheng, H. K. Renawala, W. P. Wuelfing, N. Buist, I. Raheem, A. Cote, J. C. Givand, S. B. Gabelli, R. Burlage, A. C. Templeton, G. Hu, Y. Su, Protein stability and viscosity in molecularly crowded high- concentration biologics. Adv. Drug Deliv. Rev. 233, 115854 (2026)

  32. [32]

    T.-S. Wong, S. H. Kang, S. K. Y. Tang, E. J. Smythe, B. D. Hatton, A. Grinthal, J. Aizenberg, Bioinspired Self-Repairing Slippery Surfaces with Pressure-Stable Omniphobicity. Nature 477, 443–447 (2011)

  33. [33]

    Jayaprakash, M

    V. Jayaprakash, M. Costalonga, S. Dhulipala, K. K. Varanasi, Enhancing the injectability of high concentration drug formulations using core annular flows. Adv. Healthc. Mater. 9, 2001022 (2020)

  34. [34]

    B. R. Solomon, K. S. Khalil, K. K. Varanasi, Drag Reduction Using Lubricant- Impregnated Surfaces in Viscous Laminar Flow. Langmuir 30, 10970–10976 (2014)

  35. [35]

    B. R. Solomon, X. Chen, L. Rapoport, A. Helal, G. H. McKinley, Y.-M. Chiang, K. K. Varanasi, Enhancing the Performance of Viscous Electrode-Based Flow Batteries Using Lubricant-Impregnated Surfaces. ACS Appl. Energy Mater. 1, 3614–3621 (2018)

  36. [36]

    D. D. Joseph, and R. Bai, K. P. Chen, Y. Y. Renardy, Core-Annular Flows. Annu. Rev. Fluid Mech. 29, 65–90 (1997)

  37. [37]

    J. S. Wexler, I. Jacobi, H. A. Stone, Shear- Driven Failure of Liquid-Infused Surfaces. Phys. Rev. Lett. 114, 168301 (2015)

  38. [38]

    Dunne, T

    P. Dunne, T. Adachi, A. A. Dev, A. Sorrenti, L. Giacchetti, A. Bonnin, C. Bourdon, P. H. Mangin, J. M. D. Coey, B. Doudin, T. M. Hermans, Liquid flow and control without solid walls. Nature 581, 58–62 (2020)

  39. [39]

    A. A. Dev, P. Dunne, T. M. Hermans, B. Doudin, Fluid Drag Reduction by Magnetic Confinement. Langmuir, doi: 10.1021/acs.langmuir.1c02617 (2022)

  40. [40]

    A. A. Dev, G. Bagheri, E. Bodenschatz, T. M. Hermans, B. Doudin, Suppressing Interfacial Instability of Immiscible Liquid- in-Liquid Flow Using Magnetic Forces. Adv. Sci. 13, e10327 (2026)

  41. [41]

    L. M. Stancanelli, E. Secchi, M. Holzner, Magnetic fluid film enables almost complete drag reduction across laminar and turbulent flow regimes. Commun. Phys. 7, 30 (2024)

  42. [42]

    Goyon, A

    J. Goyon, A. Colin, L. Bocquet, How does a soft glassy material flow: finite size effects, non local rheology , and flow cooperativity. Soft Matter 6, 2668–2678 (2010)

  43. [43]

    Jamali, Multiscale Nature of Thixotropy and Rheological Hysteresis in Attractive Colloidal Suspensions under Shear

    S. Jamali, Multiscale Nature of Thixotropy and Rheological Hysteresis in Attractive Colloidal Suspensions under Shear. Phys. Rev. Lett. 123 (2019)

  44. [44]

    A. A. Dev, T. M. Hermans, B. Doudin, Ultra-Soft Liquid-Ferrofluid Interfaces. Adv. Funct. Mater. 34, 2411811 (2024)