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arxiv: 2204.13052 · v3 · pith:EBAX2Y55 · submitted 2022-04-27 · cond-mat.mtrl-sci · cond-mat.mes-hall

Hidden interplay of current-induced spin and orbital torques in bulk Fe₃GeTe₂

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classification cond-mat.mtrl-sci cond-mat.mes-hall
keywords torquesorbitalmaterialspropertiesspinspin-orbittorquewaals
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Low crystal symmetry of magnetic van der Waals materials naturally promotes spin-orbital complexity unachievable in common magnetic materials used for spin-orbit torque switching. Here, using first-principles methods, we demonstrate that an interplay of spin and orbital degrees of freedom has a profound impact on spin-orbit torques in a prototype van der Waals ferromagnet: Fe$_3$GeTe$_2$ (FGT). While we show that bulk FGT hosts strong "hidden" current-induced torques harvested by each of its layers, we uncover that their origin alternates between the conventional spin flux torque and the so-called orbital torque as the magnetization direction is varied. A drastic difference in the behavior of the two types of torques results in a non-trivial evolution of switching properties with doping. Our findings promote the design of non-equilibrium orbital properties as the guiding mechanism for crafting the properties of spin-orbit torques in layered van der Waals materials.

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