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Imaging inter-valley coherent order in magic-angle twisted trilayer graphene

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arxiv 2304.10586 v1 pith:GSHCDVEH submitted 2023-04-20 cond-mat.str-el

classification cond-mat.str-el
keywords phasescorrelatedmoirgrapheneinter-valleykekulmattgrange
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Magic-angle twisted trilayer graphene (MATTG) exhibits a range of strongly correlated electronic phases that spontaneously break its underlying symmetries. The microscopic nature of these phases and their residual symmetries stands as a key outstanding puzzle whose resolution promises to shed light on the origin of superconductivity in twisted materials. Here we investigate correlated phases of MATTG using scanning tunneling microscopy and identify striking signatures of interaction-driven spatial symmetry breaking. In low-strain samples, over a filling range of about 2-3 electrons or holes per moir\'e unit cell, we observe atomic-scale reconstruction of the graphene lattice that accompanies a correlated gap in the tunneling spectrum. This short-scale restructuring appears as a Kekul\'e supercell -- implying spontaneous inter-valley coherence between electrons -- and persists in a wide range of magnetic fields and temperatures that coincide with the development of the gap. Large-scale maps covering several moir\'e unit cells further reveal a slow evolution of the Kekul\'e pattern, indicating that atomic-scale reconstruction coexists with translation symmetry breaking at the much longer moir\'e scale. We employ auto-correlation and Fourier analyses to extract the intrinsic periodicity of these phases and find that they are consistent with the theoretically proposed incommensurate Kekul\'e spiral order. Moreover, we find that the wavelength characterizing moir\'e-scale modulations monotonically decreases with hole doping away from half-filling of the bands and depends only weakly on the magnetic field. Our results provide essential insights into the nature of MATTG correlated phases in the presence of strain and imply that superconductivity emerges from an inter-valley coherent parent state.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Fractional Chern mosaic in supermoir\'e graphene

    cond-mat.str-el 2024-11 conditional novelty 7.0 of 10

    Helical trilayer graphene with momentum-dependent tunneling is predicted to host a fractional Chern mosaic at filling 3+1/3: local fractional Chern insulators whose fractionalization pattern varies on the supermoiré scale.

  2. Nanoscale infrared and microwave imaging of stacking faults in multilayer graphene

    cond-mat.mes-hall 2025-04 conditional novelty 6.0 of 10

    AFM-IR and sMIM can distinguish Bernal, rhombohedral, and intermediate stacking orders in multilayer graphene, including under a boron nitride coating.

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