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Magnetic phase diagram of a two-orbital model for bilayer nickelates varying doping

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arxiv 2408.05689 v1 pith:NCLUH5PI submitted 2024-08-11 cond-mat.str-el

classification cond-mat.str-el
keywords couplingmagnetictimes2antiferromagneticbilayerobtainedplanestate
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abstract

Motivated by the recently discovered high-$T_c$ bilayer nickelate superconductor La$_3$Ni$_2$O$_7$, we comprehensively research a bilayer $2\times2\times2$ cluster for different electronic densities $n$ by using the Lanczos method. We also employ the random-phase approximation to quantify the first magnetic instability with increasing Hubbard coupling strength, also varying $n$. Based on the spin structure factor $S(q)$, we have obtained a rich magnetic phase diagram in the plane defined by $n$ and $U/W$, at fixed Hund coupling. We have observed numerous states, such as A-AFM, Stripes, G-AFM, and C-AFM. For half-filling $n=2$ (two electrons per Ni site, corresponding to $N$ = 16 electrons), the canonical superexchange interaction leads to a robust G-AFM state $(\pi,\pi,\pi)$ with antiferromagnetic couplings in plane and between layers. By increasing or decreasing electronic densities, ferromagnetic tendencies emerge from the ``half-empty'' and ``half-full'' mechanisms, leading to many other interesting magnetic tendencies. In addition, the spin-spin correlations become weaker both in the hole or electron doping regions compared with half-filling. At $n = 1.5$ (or $N=12$), density corresponding to La$_3$Ni$_2$O$_7$, we obtained the ``Stripe 2'' ground state (antiferromagnetic coupling in one in-plane direction, ferromagnetic coupling in the other, and antiferromagnetic coupling along the $z$-axis) in the $2\times2\times2$ cluster. In addition, we obtained a much stronger AFM coupling along the $z$-axis than the magnetic coupling in the $xy$ plane. The random-phase approximation calculations with varying $n$ give very similar results as Lanczos. Meanwhile, a state with $q/\pi = (0.6, 0.6, 1)$ close to the E-phase wavevector is found in our RPA calculations by slightly reducing the filling to $n=1.25$, possibly responsible for the E-phase SDW recently observed in experiments.

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  1. Spin density wave and superconductivity in the bilayer $t$-$J$ model of $\rm{La}_{3}Ni_{2}O_{7}$ under renormalized mean-field theory

    cond-mat.supr-con 2024-12 conditional novelty 5.0 of 10

    A renormalized mean-field study of a bilayer t-J model predicts antiferromagnetic d-wave and double-spin-stripe s-wave coexistence states in La3Ni2O7, with the transition tuned by inter-layer coupling.

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