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arxiv 2306.10291 v2 pith:PKTYAHLA submitted 2023-06-17 cond-mat.mes-hall

Proximity-induced spin-orbit coupling in phosphorene on a WSe₂ monolayer

classification cond-mat.mes-hall
keywords phosphorenespin-orbitcouplingfieldheterostructureout-of-planesymmetrybilayer
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We investigate, using first-principles methods and effective-model simulations, the spin-orbit coupling proximity effects in a bilayer heterostructure comprising phosphorene and WSe$_2$ monolayers. We specifically analyze holes in phosphorene around the $\Gamma$ point, at which we find a significant increase of the spin-orbit coupling that can be attributed to the strong hybridization of phosphorene with the WSe$_2$ bands. We also propose an effective spin-orbit model based on the ${\bf C}_{1{\rm v}}$ symmetry of the studied heterostructure. The corresponding spin-orbit field can be divided into two parts: the in-plane field, present due to the broken nonsymmorphic horizontal glide mirror plane symmetry, and the dominant out-of-plane field triggered by breaking the out-of-plane rotational symmetry of the phosphorene monolayer. Furthermore, we also demonstrate that a heterostructure with 60$^\circ$ twist angle exhibits an opposite out-of-plane spin-orbit field, indicating that the coupling can effectively be tuned by twisting. The studied phosphorene/WSe$_2$ bilayer is a prototypical low common-symmetry heterostructure in which the proximity effect can be used to engineer the spin texture of the desired material.

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