pith:X5DO7YIV
Optically detected nuclear magnetic resonance of carbon-13 in bulk diamond
Landau-Zener microwave sweeps enable optical polarization and readout of large 13C nuclear spin ensembles in diamond.
arxiv:2605.00152 v2 · 2026-04-30 · quant-ph · cond-mat.mes-hall · physics.atom-ph · physics.ins-det · physics.optics
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Claims
We demonstrate a technique that allows for both optical polarization and readout of large ensembles of ~10^{16} polarized nuclear spins... realize a nuclear-spin-dependent fluorescence contrast exceeding 0.5% peak-to-peak. We observe nuclear spin dephasing times T2*~2 ms that only modestly improve with homonuclear dipolar decoupling, indicating that they are limited by the longitudinal spin relaxation of nearby NV electron spins.
The assumption that the observed fluorescence contrast arises specifically from remote 13C nuclear spins via efficient bidirectional Landau-Zener transfer and that T2* is limited by NV relaxation rather than other unaccounted mechanisms or sample variations.
A microwave-sweep technique using Landau-Zener transitions transfers polarization between NV electron spins and remote 13C nuclei, enabling optically detected NMR with >0.5% contrast and ~2 ms T2* in natural-abundance diamond.
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| First computed | 2026-06-02T01:03:47.764889Z |
|---|---|
| Builder | pith-number-builder-2026-05-17-v1 |
| Signature | Pith Ed25519
(pith-v1-2026-05) · public key |
| Schema | pith-number/v1.0 |
Canonical hash
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Canonical record JSON
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