Coupled modeling of crack electrolyte wetting in battery particles reveals 8x reaction flux amplification at crack tips and shows that uniform-flux assumptions systematically underpredict capacity and stress by 25% and 10% respectively.
Xu, Electrolytes and interphases in li-ion batterie s and beyond, Chemical reviews 114 (23) (2014) 11503–11618
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On the role of crack electrolyte wetting in the degradation and performance of battery active particles
Coupled modeling of crack electrolyte wetting in battery particles reveals 8x reaction flux amplification at crack tips and shows that uniform-flux assumptions systematically underpredict capacity and stress by 25% and 10% respectively.