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arxiv: 1904.08615 · v1 · pith:QJKOX5DQnew · submitted 2019-04-18 · ❄️ cond-mat.mtrl-sci · cond-mat.str-el

Suppression of long range magnetic ordering and electrical conduction in Y_(1.7)Bi_(0.3)Ir₂O₇ thin film

classification ❄️ cond-mat.mtrl-sci cond-mat.str-el
keywords magneticconductionelectricalfilmorderingstatesthinabsent
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We find that the long-range magnetic ordering is absent and electrical conduction suppressed in Y$_{1.7}$Bi$_{0.3}$Ir$_2$O$_7$/YSZ(100) thin film prepared by pulsed laser deposition. The sharp down-turn of inverse magnetic susceptibility X-1(T) from the conventional Curie-Weiss behaviour below T* ~ 168K suggests an inhomogeneous ferromagnetic Griffiths like phase. The transport and magnetic properties are explained on the basis of the coexistence of mixed oxidation states of Ir, (i.e. Ir4+ and Ir3+) leading to non-magnetic defects and reduction in t2g density of states at the Fermi level.

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