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arxiv 2012.12777 v3 pith:YDPEJU5H submitted 2020-12-23 cond-mat.mtrl-sci

Effect of Fullerene on domain size and relaxation in a perpendicularly magnetized Pt/Co/C60/Pt system

classification cond-mat.mtrl-sci
keywords systemdomainspinterfaceanisotropypolarizedsizespindynamics
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Buckminsterfullerene (C60) can exhibit ferromagnetism at the interface (called as a spinterface) when it is placed next to a ferromagnet (FM). Formation of such spinterface happens due to orbital hybridization and spin polarized charge transfer at the interface. The spinterface can influence the domain size and dynamics of the organic/ferromagnetic heterostructure. Here, we have performed magnetic domain imaging and studied the relaxation dynamics in Pt/Co/C60/Pt system with perpendicular anisotropy. We have compared the results with its parent Pt/Co/Pt system. It is observed that presence of C60 in the Pt/Co/Pt system increases the anisotropy and a decrease in the bubble domain size. Further the switching time of Pt/Co/C60/Pt system is almost two times faster than Pt/Co/Pt system. We have also performed the spin polarized density functional theory (DFT) calculations to understand the underneath mechanism. DFT results show formation of a spin polarized spinterface which leads to an enhancement in anisotropy.

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