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arxiv: 2305.07734 · v1 · pith:N6ZXTLXPnew · submitted 2023-05-12 · ❄️ cond-mat.str-el

Disorder-enriched magnetic excitations in the Kitaev quantum spin liquid candidate Na₂Co₂TeO₆

classification ❄️ cond-mat.str-el
keywords magneticexcitationsspindisorderkitaevliquidmodesquantum
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Using optical magneto-spectroscopy, we investigate the magnetic excitations of Na$_2$Co$_2$TeO$_6$ in a broad magnetic field range ($0\ \rm{T}\leq B\leq 17.5\ \rm{T}$) at low temperature. Our measurements reveal rich spectra of in-plane magnetic excitations with a surprisingly large number of modes, even in the high-field spin-polarized state. Theoretical calculations find that the Na-occupation disorder in \NCTO plays a crucial role in generating these modes. Our work demonstrates the necessity to consider disorder in the spin environment in the search for Kitaev quantum spin liquid states in practicable materials.

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