Modulated conjugation as a means for attaining a record high intrinsic hyperpolarizability
classification
⚛️ physics.chem-ph
physics.optics
keywords
conjugationhyperpolarizabilityintrinsicmodulatedacceptorapparentattainingbeen
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We report on a series of chromophores that have been synthesized with a modulated conjugation path between donor and acceptor. Hyper-Rayleigh scattering measurements of the best molecule show an enhanced intrinsic hyperpolarizability that breaches the apparent limit of all previously studied molecules.
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