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Three-dimensional mapping of the altermagnetic spin splitting in CrSb

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arxiv 2405.12575 v3 pith:DNQEFKVJ submitted 2024-05-21 cond-mat.mtrl-sci cond-mat.str-el

classification cond-mat.mtrl-scicond-mat.str-el
keywords splittingaltermagneticspinfermilargelevelneararpes
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Altermagnetism, a kind of collinear magnetism that is characterized by a momentum-dependent band and spin splitting without net magnetization, has recently attracted considerable interest. Finding altermagnetic materials with large splitting near the Fermi level necessarily requires three-dimensional k-space mapping. While this is crucial for spintronic applications and emergent phenomena, it remains challenging. Here, using synchrotron-based angle-resolved photoemission spectroscopy (ARPES), spin-resolved ARPES and model calculations, we uncover a large altermagnetic splitting, up to ~1.0 eV, near the Fermi level in CrSb. We verify its bulk-type g-wave altermagnetism through systematic three-dimensional k-space mapping, which unambiguously reveals the altermagnetic symmetry and associated nodal planes. Spin-resolved ARPES measurements further verify the spin polarizations of the split bands near Fermi level. Tight-binding model analysis indicates that the large altermagnetic splitting arises from strong third-nearest-neighbor hopping mediated by Sb ions. The large band/spin splitting near Fermi level in metallic CrSb, together with its high TN (up to 705 K) and simple spin configuration, paves the way for exploring emergent phenomena and spintronic applications based on altermagnets.

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Cited by 5 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Persistent spin currents in superconducting altermagnets

    cond-mat.supr-con 2025-07 conditional novelty 7.0 of 10

    Model calculations show that superconducting altermagnets can support persistent spin-polarized and pure spin supercurrents that survive spin-orbit coupling and magnetic disorder.

  2. Elasto-Hall conductivity and the anomalous Hall effect in altermagnets

    cond-mat.mtrl-sci 2025-02 accept novelty 7.0 of 10

    Strain distorts the Berry curvature quadrupole of an altermagnet into a net monopole, producing an anomalous Hall effect linear in the electric field.

  3. N\'eel vector-dependent anomalous transport in altermagnetic metal CrSb

    cond-mat.mtrl-sci 2024-12 conditional novelty 6.0 of 10

    First-principles calculations predict that CrSb shows a Neel-vector-dependent anomalous Hall conductivity up to 72 S/cm and a room-temperature anomalous Nernst conductivity of -0.19 A/m/K, both maximal when the Neel v...

  4. Transport theory and spin-transfer physics in d-wave altermagnets

    cond-mat.mes-hall 2024-12 conditional novelty 5.0 of 10

    The authors derive from a microscopic t-J model a mesoscale transport theory in which charge currents exert transverse spin-transfer torques, enabling current-driven domain-wall motion in d-wave altermagnets.

  5. Symmetry, microscopy and spectroscopy signatures of altermagnetism

    cond-mat.mtrl-sci 2025-06 unverdicted

    A review of the symmetry, microscopic origin, and detection of altermagnetism, a collinear magnetic phase with alternating spin polarization in momentum space.

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