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Roadmap for Quantum Nanophotonics with Free Electrons

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arxiv 2503.14678 v2 pith:6MTRAKAP submitted 2025-03-18 cond-mat.mes-hall physics.app-phphysics.optics

classification cond-mat.mes-hallphysics.app-phphysics.optics
keywords quantumelectronelectronsfreecarrycontrolfieldinformation
verification ladder T0 review T1 audit T2 compute T3 formal

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Over the past century, continuous advancements in electron microscopy have enabled the synthesis, control, and characterization of high-quality free-electron beams. These probes carry an evanescent electromagnetic field that can drive localized excitations and provide high-resolution information on material structures and their optical responses, currently reaching the sub-{\aa}ngstr\"om and few-meV regime. Moreover, combining free electrons with pulsed light sources in ultrafast electron microscopy adds temporal resolution in the sub-femtosecond range while offering enhanced control of the electron wave function. Beyond their exceptional capabilities for time-resolved spectromicroscopy, free electrons are emerging as powerful tools in quantum nanophotonics, on par with photons in their ability to carry and transfer quantum information, create entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena. This Roadmap outlines the current state of this rapidly evolving field, highlights key challenges and opportunities, and discusses future directions through a collection of topical sections prepared by leading experts.

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Cited by 4 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Ghost Imaging with Free Electron-Photon Pairs

    quant-ph 2025-09 conditional novelty 7.0 of 10

    First demonstration of two-dimensional ghost imaging using electron-photon pairs in a TEM, achieving 2 micrometer resolution on complex patterns.

  2. Wave-mixing cathodoluminescence microscopy of low-frequency excitations

    cond-mat.mes-hall 2025-08 unverdicted novelty 7.0 of 10

    Visible light can be inelastically scattered by an electron's evanescent field through a specimen's second-order nonlinearity, shifting the photon energy by the specimen's low-frequency vibrational mode.

  3. Spin Squeezing in Electron Microscopy

    quant-ph 2025-07 conditional novelty 7.0 of 10

    Spin squeezing of free electrons in a Mach-Zehnder interferometer is proposed as a way to push phase measurement accuracy in electron microscopy below the shot-noise limit.

  4. Quantum sensing of electron beams using solid-state spins

    quant-ph 2025-08 conditional novelty 6.0 of 10

    A bunched electron beam is shown to be a viable probe of diamond NV spin ensembles, with T1 relaxometry placing an upper bound on the free-electron-spin coupling strength.

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