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Roadmap for Quantum Nanophotonics with Free Electrons
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Over the past century, continuous advancements in electron microscopy have enabled the synthesis, control, and characterization of high-quality free-electron beams. These probes carry an evanescent electromagnetic field that can drive localized excitations and provide high-resolution information on material structures and their optical responses, currently reaching the sub-{\aa}ngstr\"om and few-meV regime. Moreover, combining free electrons with pulsed light sources in ultrafast electron microscopy adds temporal resolution in the sub-femtosecond range while offering enhanced control of the electron wave function. Beyond their exceptional capabilities for time-resolved spectromicroscopy, free electrons are emerging as powerful tools in quantum nanophotonics, on par with photons in their ability to carry and transfer quantum information, create entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena. This Roadmap outlines the current state of this rapidly evolving field, highlights key challenges and opportunities, and discusses future directions through a collection of topical sections prepared by leading experts.
Forward citations
Cited by 4 Pith papers
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Ghost Imaging with Free Electron-Photon Pairs
First demonstration of two-dimensional ghost imaging using electron-photon pairs in a TEM, achieving 2 micrometer resolution on complex patterns.
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Wave-mixing cathodoluminescence microscopy of low-frequency excitations
Visible light can be inelastically scattered by an electron's evanescent field through a specimen's second-order nonlinearity, shifting the photon energy by the specimen's low-frequency vibrational mode.
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Spin Squeezing in Electron Microscopy
Spin squeezing of free electrons in a Mach-Zehnder interferometer is proposed as a way to push phase measurement accuracy in electron microscopy below the shot-noise limit.
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Quantum sensing of electron beams using solid-state spins
A bunched electron beam is shown to be a viable probe of diamond NV spin ensembles, with T1 relaxometry placing an upper bound on the free-electron-spin coupling strength.
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