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arxiv: 1312.2357 · v4 · pith:6M4CZU22new · submitted 2013-12-09 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

Spectroscopic study of the magnetic ground state of Nb_(1-y)Fe_(2+y)

classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords magneticorderspinbulkferromagnetismnbfestateamplitudes
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We have investigated single crystals and polycrystals from the series Nb$_{1-y}$Fe$_{2+y}$, $-0.004 \leq y \leq 0.018$ by electron spin resonance, muon spin relaxation and M\"ossbauer spectroscopy. Our data establish that at lowest temperatures all samples exhibit bulk magnetic order. Slight Fe-excess induces low-moment ferromagnetism, consistent with bulk magnetometry ($\simeq 0.06 ~\mu_B/{\rm Fe}$), Nb--rich and stoichiometric NbFe$_2$ display spin density wave order with small magnetic moment amplitudes of the order $\sim 0.001 - 0.01 ~\mu_B/{\rm Fe}$. This provides microscopic evidence for a modulated magnetic state on the border of ferromagnetism in NbFe$_2$.

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