Not yet reviewed by Pith; the record is open.

Maximization saturation magnetic induction (Bs) of soft magnetic alloys is essential for the high power-density electromagnetic devices. However, identifying the alloy compositions with high Bs often replies on the lab-intensive melt casting method and a high-throughput characterization on magnetic properties remains challenging. Here, we develop a new combinatorial method for fast screening alloys with optimal soft magnetic properties based on the high-throughput MOKE screening method. Based on the combinatorial method, we found that the alloys with a combination of high Bs and low coercivity (Hc) tend to have a feature of amorphous-nanocrystalline biphase microstructure. We also identified an amorphous/nanocrystalline alloy film with the composition the Fe68.09Co17.02B10.9Si4, exhibiting an ultra-high Bs up to 2.02 T that surpasses all amorphous/nanocrystalline alloys reported so far and is comparable to that of silicon steels, together with a high resistivity of 882 {\mu}{\Omega} {\dot} cm, about 17 times of silicon steels. Our high-throughput magnetic screening method provides a paradigm for understanding the relationship between microstructure and magnetic properties and the development of the next-generation soft magnetic materials.