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arxiv: 2507.10964 · v1 · pith:Z4U65YJKnew · submitted 2025-07-15 · ❄️ cond-mat.mtrl-sci · cond-mat.str-el

Weak low-temperature ferromagnetism and linear magnetoresistance in Lu_(0.75)Fe₆Sn₆ with a disordered HfFe₆Ge₆-type structure

classification ❄️ cond-mat.mtrl-sci cond-mat.str-el
keywords structureferromagnetismmagneticweakab-planedisorderhffelinear
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We report the synthesis of Lu$_{0.75}$Fe$_6$Sn$_6$ single crystals with a Fe-kagome lattice using a self-flux method. The crystal structure, magnetic, thermodynamic and electrical transport properties were investigated. Structure refinement reveals that Lu$_{0.75}$Fe$_6$Sn$_6$ has a HfFe$_6$Ge$_6$-type structure as the major framework intergrown with a CoSn-type structure, leading to a vacancy of 25% on the Lu-site and disorder on the Sn-site. It exhibits a significant magnetic anisotropy with weak ferromagnetism in the ab-plane below 40 K and antiferromagnetic behavior along the c-axis. The weak ferromagnetism is due to the canted antiferromagnetism with magnetic moment deviating from the $c$-axis to the ab-plane. Besides, an anisotropic non-saturated linear magnetoresistance is also observed in Lu$_{0.75}$Fe$_6$Sn$_6$, probably resulting from the structural disorder in the sample.

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