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Electrically controlled heat transport in multilayer graphene
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The ability to control heat transport with electrical signals has been an outstanding challenge due to the lack of efficient electrothermal materials. Previous attempts have mainly concentrated on phase-change and layered materials and encountered various problems such as low thermal conductivities and modest on/off ratios. Here, we demonstrate a graphene-based electrothermal switch enabling electrically tuneable heat flow. The device uses reversible electro-intercalation of ions to modulate the in-plane thermal conductivity of graphene film by over thirteen-fold via electrically tuneable phonon scattering. We anticipate that our results could provide a realistic pathway for adaptive thermal transport enabling a new class of electrically driven thermal devices which would find a broad spectrum of applications in aerospace and microelectronics.
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